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Not really. I've been to several dozen countries. While there were places I enjoyed significantly more than others, I don't think I have any major regrets or complaints. I was incredibly disappointed by Athens - it was such a filthy and rotten city, and that's coming from somebody who's enjoyed a lot of countries less developed than Greece.
But I wouldn't "take back" that excursion if I could. Likewise, while Iceland was beautiful, I don't view it as being a very memorable place. Again, though, I'm happy I went and still have lots of good memories of hitchhiking, making new friends, and seeing a unique place.